Graphical abstract of scientific publication.

A. Davis,♦ K. Parui,♦ A. M. M. Hasan, L. A. Pineda, J. D. Langhout, K. A. Treaster, M. M. Butala,* A. M. Evans.* Cross-linking organic cathodes enhances stability at the expense of ionic accessibility. J. Mater. Chem. A, 12 (2024) 28874-28881. (♦ equal contribution)